Charge density wave interlayer correlations in 1T-TaS2

DOI

This proposal aims to study the microscopic stabilization mechanism of different charge density wave stacking schemes in the layered material 1T-TaS2. This material has a complex electronic phase diagram as a function of pressure and temperature which exhibits various CDW phases along with pressure induced superconductivity. X-ray diffraction (XRD) experiments have shown that not only the in-plane CDW order changes as a function of pressure and temperature, but also the stacking order of the CDW in the out-of-plane direction is affected. DFT simulations have identified S-3pz derived bounding states as central players in stabilizing the different stacking schemes in this material. However, direct experimental evidence for such a mechanism is yet to be found. Therefore, we propose to use the newly created possibilities at ID12 to study the behaviour of exactly these S-3pz states as a function of pressure and temperature by means of Xray-absorption near edge spectroscopy (XANES).

Identifier
DOI https://doi.org/10.15151/ESRF-ES-1915450426
Metadata Access https://icatplus.esrf.fr/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatplus.esrf.fr:inv/1915450426
Provenance
Creator Steven GEBEL ORCID logo; SWARNAMAYEE MISHRA ORCID logo; Tobias RITSCHEL; Fabrice WILHELM ORCID logo
Publisher ESRF (European Synchrotron Radiation Facility)
Publication Year 2027
Rights CC-BY-4.0; https://creativecommons.org/licenses/by/4.0
OpenAccess true
Representation
Resource Type Data from large facility measurement; Collection
Discipline Particles, Nuclei and Fields