Structural Determination of Novel Ytterbium Polyhydrides

DOI

Dense lanthanide polyhydrides are theorised to be promising candidates to exhibit high-temperature superconductivity, expedited by the observation of superconductivity in the La-H system. The heavy lanthanides have electronic properties which are thought to enhance superconductivity in hydrides, however, there remain systems that have yet to be fully explored, such as Yb-H. In our preliminary experiments on the Yb-H system, we observe the formation of two novel polyhydrides: Yb4H23 and YbH7.5, synthesised at pressures exceeding 150 GPa and temperatures above 1000 K. Here, we propose to comprehensively study the Yb-H system, establishing phase stability, determining the equations of state and exploring further hydrogenation. This is imperative to our parallel studies investigating their electronic transport properties.

Identifier
DOI https://doi.org/10.15151/ESRF-ES-1883533213
Metadata Access https://icatplus.esrf.fr/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatplus.esrf.fr:inv/1883533213
Provenance
Creator Hannah SHUTTLEWORTH ORCID logo; Samuel GALLEGO PARRA ORCID logo; Israel OSMOND ORCID logo; Mikhail KUZOVNIKOV; Ross HOWIE ORCID logo
Publisher ESRF (European Synchrotron Radiation Facility)
Publication Year 2027
Rights CC-BY-4.0; https://creativecommons.org/licenses/by/4.0
OpenAccess true
Representation
Resource Type Data from large facility measurement; Collection
Discipline Particles, Nuclei and Fields