Enabling deep understanding of Power-to-Ammonia catalysts for renewable fuel production with the help of transient operando photon-in/photon

DOI

This LTP is motivated by systematic studies on ammonia synthesis catalysts under the realistic conditions of the Haber-Bosch process, as employed for the production of sustainable renewable ammonia at offshore wind power plants. Over the course of 6 beamtime scheduling periods, electronic and geometric structure of active metals (Fe, Ru) as well as of electronic (K, Cs, Ca, Ba) and structural (Al, Si) promoters will be thoroughly studied at the ID26 beamline under stationary and transient conditions. In the course of the LTP a pixel detector will be installed in the TEXS which, together with sets of high quality Johansson crystals, which will enable X-ray Fluorescence Intensity Ratio Detection (XFIRD). Furthermore, a high pressure operando catalysis cell will be developed. The planned investments will enable spatially- and time-resolved operando tender X-ray HERFD-XANES and XES spectroscopy on working catalysts for chemical energy storage and related processes.

Identifier
DOI https://doi.org/10.15151/ESRF-ES-2220632617
Metadata Access https://icatplus.esrf.fr/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatplus.esrf.fr:inv/2220632617
Provenance
Creator Samuel STRUZEK; VASYL MARCHUK ORCID logo; Jan-Dierk GRUNWALDT ORCID logo; Jennifer KLAUCKE ORCID logo; Maria CASAPU; Tomás VERGARA ORCID logo
Publisher ESRF (European Synchrotron Radiation Facility)
Publication Year 2028
Rights CC-BY-4.0; https://creativecommons.org/licenses/by/4.0
OpenAccess true
Representation
Resource Type Data from large facility measurement; Collection
Discipline Particles, Nuclei and Fields