XAS/XES probing chemical evolution in Solid-state Cl-ion batteries with conversion electrodes

DOI

This project aims to study the redox mechanism of composite electrodes in solid-state chloride-ion batteries (CIBs) via tender x-ray absorption/emission spectroscopy. By using solid cells with composite electrodes as samples, the emission lines and the absorption spectra can be measured on Cl K-edge and the respective metal edges, allowing us to probe the redox-active species and their evolution at different charge states and cycles. In combination with other complementary techniques, we want to understand the fundamental mechanism of the conversion reactions for these metal chloride electrodes, and to identify the factors hindering the reversibility and stability in prolonged cycles. The findings will provide a valuable guidance on the selection of metal chloride cathodes, and help the rational design and optimization of CIBs for enhanced energy/power density and cycle life.

Identifier
DOI https://doi.org/10.15151/ESRF-ES-2232212118
Metadata Access https://icatplus.esrf.fr/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatplus.esrf.fr:inv/2232212118
Provenance
Creator OLGA FILIMONOVA ORCID logo; Hui WANG; Yang HU ORCID logo; Soutam PANJA ORCID logo
Publisher ESRF (European Synchrotron Radiation Facility)
Publication Year 2028
Rights CC-BY-4.0; https://creativecommons.org/licenses/by/4.0
OpenAccess true
Representation
Resource Type Data from large facility measurement; Collection
Discipline Particles, Nuclei and Fields