Studies of local order and clustering in (1-x)BaTiO3-xBiYbO3 Perovskites

DOI

We propose total scattering experiments on samples of (1-x)BaTiO3-xBiYbO3 perovskites with x = 0, 0.04, 0.08 and 0.15 to resolve issues over the local structure and degree of clustering of the dopant system. The simultaneous incorporation of Bi3+ and Yb3+ into the BaTiO3 lattice leads to a continuous reduction in tetragonality based on powder X-ray diffraction data and disappearance of long-range ferroelectric polarisation as indicated by Raman spectroscopy. However, the Raman spectra for x > 0.06 provide strong evidence for the occurrence of short-range deformations and local non-cubic structure and this leads to dielectric behaviour that is different than expected for a perovskite with an average crystal symmetry described by the cubic centrosymmetric Pm-3m space group. Analysis of total scattering data will resolve how the local structure is leading to the dielectric behaviour.

Identifier
DOI https://doi.org/10.5286/ISIS.E.24088352
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/24088352
Provenance
Creator Dr Joe Hriljac; Mr Tim Lucas; Mr Luke Luisman; Dr Antonio Feteira
Publisher ISIS Neutron and Muon Source
Publication Year 2014
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2011-11-27T17:58:54Z
Temporal Coverage End 2011-11-30T08:25:34Z