Order-disorder transitions in ternary unfilled skutterudites

DOI

The aim of this proposal is to study the thermal evolution of the structure of two ternary ordered skutterudites, CoGe1.5Q1.5 (Q = S, Te). At room temperature, ordering of the Ge and Q atoms results in a lowering of the symmetry of the skutterudite from cubic (Im-3) to rhombohedral (R-3). The degree of ordering is dependent on the rate of cooling of the materials, suggesting that a transition to a cubic disordered skutterudite takes place at elevated temperatures. Given the small deviation of the rhombohedral angle from 90º found for these phases, high-resolution data are essential and therefore we propose to use HRPD. In addition, we are seeking to investigate ordering at the metal site for the ternary skutterudite Fe0.5Ni0.5Sb3.

Identifier
DOI https://doi.org/10.5286/ISIS.E.24083805
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/24083805
Provenance
Creator Professor Anthony Powell; Dr Paz Vaqueiro-Rodriguez; Dr Andreas Kaltzoglou
Publisher ISIS Neutron and Muon Source
Publication Year 2014
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2011-04-07T07:45:49Z
Temporal Coverage End 2011-07-18T05:45:07Z