Increasing Oxide Ion Vacancy Concentration Bi2O3 Based Electrolytes through di-substitution

DOI

Recent research has shown that bismuth oxide based electrolytes are viable components in solid oxide fuel cells. Di-substitution of Bi3+ by an isovalent and a subvalent cation leads to stabilisation of the highly conducting fluorite delta-phase of Bi2O3. This leads to a system with nominally higher vacancy concentration than Bi2O3 itself, with higher stability than the mono-substituted systems. The present proposal seeks to investigate the oxide ion distribution in the Bi2O3-PbO-Er2O3 system and its thermal variation, with a view to explaining its conductivity behaviour. While the long range structure will be examined by conventional Rietveld analysis, a total scattering study will be carried out on the Yb substituted analogue to yield information on local structure and vacancy ordering.

Identifier
DOI https://doi.org/10.5286/ISIS.E.24091144
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/24091144
Provenance
Creator Dr Isaac Abrahams; Dr Steve Hull; Professor Franciszek Krok; Dr Stefan Norberg; Dr Marzena Leszczynska-Redek; Dr Anna Borowska; Dr Marcin Malys; Mr Ken Watson
Publisher ISIS Neutron and Muon Source
Publication Year 2016
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2013-09-18T23:00:00Z
Temporal Coverage End 2013-09-21T23:00:00Z