Probing the local magnetic structure and magnetic ground states in strongly spin-orbit coupled Iridates

DOI

Strong spin-orbit coupling often leads to exotic properties in otherwise a well understood pool of 'paramagnetic' heavy ion oxides. For a 5d4 system a J=0 total angular momentum ground state should be realised in a jj coupling scheme, which has not been observed till today. This is due to a subtle balance between electronic repulsion, crystal field (CF) and SOC, which makes the J=0 state a fragile one and also because in some cases singlet-triplet excitations of pseudospins may be at play. These excitations give rise to tiny magnetic moments which owing to exchange interactions on geometrically frustrated lattices may give rise to spin-orbital liquid state. We propose to probe with muSR such frustrated 5d4 iridate compounds having variations in the crystal field, based on the local Iridium coordination and overall crystal lattice.

Identifier
DOI https://doi.org/10.5286/ISIS.E.82352754
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/82352754
Provenance
Creator Professor Philippe Mendels; Dr Sugata Ray; Mr Abhishek Nag; Professor Fabrice Bert; Dr Aidy Hillier; Dr Edwin Kermarrec; Mr Rafikul Ali Saha
Publisher ISIS Neutron and Muon Source
Publication Year 2019
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Natural Sciences; Physics
Temporal Coverage Begin 2016-10-01T08:30:00Z
Temporal Coverage End 2016-10-04T08:30:00Z