Quasiparticle interference on the surface of Bi<sub>2</sub>Se<sub>3</sub> terminated (PbSe)<sub>5</sub>(Bi<sub>2</sub>Se<sub>3</sub>)<sub>6</sub>

DOI

Among the family of topological superconductors derived from Bi<sub>2</sub>Se<sub>3</sub>, Cu<sub>x</sub>(PbSe)<sub>5</sub>(Bi<sub>2</sub>Se<sub>3</sub>)<sub>6</sub> is unique in its surface termination of a single quintuple layer (QL) of the topological insulator (TI) Bi<sub>2</sub>Se<sub>3</sub> on an ordinary insulator PbSe. Here, we report a combined scanning tunneling microscopy (STM) and density functional theory (DFT) characterization of the cleaved surface of the parent compound (PbSe)<sub>5</sub>(Bi<sub>2</sub>Se<sub>3</sub>)<sub>6</sub> (PSBS). Interestingly, the potential disorder due to the random distribution of native defects is only Γ ∼ 4 meV, among the smallest reported for TIs. Performing high-resolution quasiparticle interference imaging (QPI) near the Fermi energy (E−E<sub>F</sub> = −1 eV to 0.6 eV) we reconstruct the dispersion relation of the dominant spectral feature and our ab initio calculations show that this surface feature originates from two bands with Rashba-like splitting due to strong spin-orbit coupling and inversion symmetry breaking. Moreover, a small hexagonal distortion of the calculated Fermi surface is seen in the full momentum space distribution of the measured scattering data. Interestingly, the scattering pattern transforms into a flower-like shape with suppressed intensity along the ΓK direction, at lower energies. However, this change is not due to the forbidden backscattering in the topological surface state in Bi<sub>2</sub>Se<sub>3</sub> but the threefold symmetry of the scattering potential itself.

This dataset contains the experimental and theoretical data of this work.

Identifier
DOI https://doi.org/10.24435/materialscloud:3c-m2
Related Identifier https://doi.org/10.5281/zenodo.7576163
Related Identifier https://doi.org/10.5281/zenodo.7284739
Related Identifier https://doi.org/10.5281/zenodo.3628250
Related Identifier https://doi.org/10.1038/s41524-020-00482-5
Related Identifier https://renkulab.io/projects/new?data=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
Related Identifier https://archive.materialscloud.org/communities/mcarchive
Related Identifier https://doi.org/10.24435/materialscloud:aj-bt
Metadata Access https://archive.materialscloud.org/oai2d?verb=GetRecord&metadataPrefix=oai_dc&identifier=oai:materialscloud.org:2470
Provenance
Creator Bagchi, Mahasweta; Rüßmann, Philipp; Bihlmayer, Gustav; Blügel, Stefan; Ando, Yoichi; Brede, Jens
Publisher Materials Cloud
Contributor Rüßmann, Philipp
Publication Year 2025
Rights info:eu-repo/semantics/openAccess; Creative Commons Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/legalcode
OpenAccess true
Contact archive(at)materialscloud.org
Representation
Language English
Resource Type info:eu-repo/semantics/other
Format text/markdown; chemical/x-cif; application/zip; text/plain; application/octet-stream
Discipline Materials Science and Engineering