Phase behaviour in lanthanum antimony niobate proton conductors

DOI

Antimony substituted lanthanum niobium oxide is a recently developed proton conductor with potential use in fuel cells, gas sensors and steam electrolysers Our preliminary work has revealed that not only does antimony substitution enhance conductivity, it also stabilizes the highly conducting scheelite phase to room temperature in contrast to the unsubstituted system which exhibits the more poorly conducting furgusonite structure at ambient temperatures. Other work suggests that the oxide ion separation distance plays a major role in determining the enthalpy of proton diffusion in these systems. A study of the correlation between electrical behaviour and oxide ion separation distance and distortion in the metal coordination environment using neutron diffraction is proposed. Details of the individual contributions of antimony and niobium will be studied using a total scattering approach.

Identifier
DOI https://doi.org/10.5286/ISIS.E.79114975
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/79114975
Provenance
Creator Ms Chuying Yu; Dr Isaac Abrahams; Dr Steve Hull; Mr Hangfeng Zhang; Dr Aleksandra Mielewczyk-Gryn; Dr Maria Gazda
Publisher ISIS Neutron and Muon Source
Publication Year 2019
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Chemistry; Natural Sciences
Temporal Coverage Begin 2016-05-05T07:00:00Z
Temporal Coverage End 2016-05-08T07:00:00Z