muSR study on a new phase in an organic charge transfer complex on a triangular lattice (C2H5)2(CH3)2Sb[Pd(dmit)2]2

DOI

We propose muSR study on magnetic properties of an organic charge transfer complex on a 2D triangular lattice, (C2H5)2(CH3)2Sb[Pd(dmit)2]2. This system has been known to exhibit charge separation forming spin-singlet below 70 K from the result of an X-ray analysis for the last decade. Our previous muSR result also revealed formation of the spin-singlet state. However, the transition temperature observed in the muSR was higher than that obtained from the X-ray analysis. Very recently, a new incommensurate phase has been found at the temperatures from 80 to 105 K, where competition between charge, spin and structural order exists, in a high-resolution X-ray diffraction measurement. The transition temperature of 105 K consists with the previous muSR result, but we have only poor data points under ZF. We will investigate magnetic state and dynamics in the newly discovered phase in detail.

Identifier
DOI https://doi.org/10.5286/ISIS.E.98003504
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/98003504
Provenance
Creator Dr Isao Watanabe; Dr Seiko Kawamura; Dr Reizo Kato; Dr Laurent Guerin
Publisher ISIS Neutron and Muon Source
Publication Year 2021
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Natural Sciences; Physics
Temporal Coverage Begin 2018-09-18T08:00:00Z
Temporal Coverage End 2018-09-20T08:21:59Z