Local Structure of Bi6WO12 and Bi28Re2O49 Oxide Ion Conductors: Role of Variable Cation Coordination

DOI

Oxide ion conductors are technologically important materials with applications in solid oxide fuel cells, oxygen sensors /pumps and membranes for oxygen separation. Two types of oxide ion conductors are well-known, those with vacancy or interstitial mechanisms. Development of new materials relies on elucidating other, more complex mechanisms of ionic mobility in solids.We request 3 day of POLARIS/GEM beam time to perform neutron total scattering/PDF work on highly disordered oxide ion conductors Bi6WO12 and Bi28Re2O49, to determine their local structures, correlate them with properties, and establish the role of W and Re variable coordination in oxide ion mobility, which is strongly suggested by our extensive preliminary work. A broader significance of this work is that it will extend the range of oxide ion conductors in which this type of ionic mobility mechanism is significant.

Identifier
DOI https://doi.org/10.5286/ISIS.E.42578714
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/42578714
Provenance
Creator Dr Matthew Tucker; Dr Mark Johnson; Professor Garry McIntyre; Dr Chris Ling; Professor Ivana Evans; Mr Matthew Tate; Miss Luiza Rosa de Araujo
Publisher ISIS Neutron and Muon Source
Publication Year 2017
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Chemistry; Natural Sciences
Temporal Coverage Begin 2014-03-01T00:00:00Z
Temporal Coverage End 2014-03-04T08:29:41Z