Moving across Pt catalysts with different size combining computations with cutting-edge X-ray spectroscopies

DOI

Pt-based heterogeneous catalysts are widely used materials for key reactions in industry like selective hydrogenations. Because of their complexity, synchrotron techniques are often used to study the active metal phase. Recent development in computational chemistry allowed for the calculation of XAS and XES spectra that can describe and possibly predict key structural and functional properties. In this context, the present study aims at acquiring top-level HERFD-XAS and resonant XES data on several Pt-based materials and create a solid experimental/simulated benchmark for spectroscopic properties involving them. A particular emphasis will be put on the size-dependency of these properties by studying a range of materials from bulk Pt to single-atom catalysts.

Identifier
DOI https://doi.org/10.15151/ESRF-ES-1872192782
Metadata Access https://icatplus.esrf.fr/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatplus.esrf.fr:inv/1872192782
Provenance
Creator Alberto RICCHEBUONO ORCID logo; VASYL MARCHUK ORCID logo; Daniele BONAVIA; Matteo SIGNORILE ORCID logo; Virginia GUIOTTO ORCID logo; Vinod PAIDI ORCID logo; Gabriele DEPLANO
Publisher ESRF (European Synchrotron Radiation Facility)
Publication Year 2027
Rights CC-BY-4.0; https://creativecommons.org/licenses/by/4.0
OpenAccess true
Representation
Resource Type Data from large facility measurement; Collection
Discipline Particles, Nuclei and Fields