Replication Data for: Chirped pulse control over the melting of superconductors

DOI

Strong field terahertz pulses are increasingly used to excite and control quantum materials at the ultrafast timescale. They have found widespread application by enabling direct addressing of the superconducting gap or Josephson resonances and are essential in Higgs spectroscopy. Large non-linear optical signals can be induced by the strong coupling of the THz and superconducting degrees of freedom. However, far less attention has been paid to the strong bidirectional coupling between field and material this implies. Here, we use the framework of the time-dependent Ginzburg-Landau equations to study the full field and material evolution of a superconductor driven by strong field terahertz pulses. We find that at high field strengths, the backreaction of the superconductor induces large changes to the driving pulse, which in turn leads to a runaway melting of the superconducting condensate. This results in a surprisingly large sensitivity to the initial driving pulse chirp, enabling these purely dynamical changes to produce order of magnitude differences in the level of melting. We also find large-scale spectral shifting of the driving pulse to occur in just a few hundred nanometers of propagation through a superconductor. We attribute these effects to an inverse plasma redshift, in which the driving field breaks Cooper pairs and decreases the free-electron mobility, analogous to reducing the density of a plasma.

Identifier
DOI https://doi.org/10.34810/data2159
Related Identifier IsSupplementTo https://doi.org/10.1103/PhysRevB.111.064513
Metadata Access https://dataverse.csuc.cat/oai?verb=GetRecord&metadataPrefix=oai_datacite&identifier=doi:10.34810/data2159
Provenance
Creator Recasens, Maria ORCID logo; Kasper, Valentin (ORCID: 0000-0001-7687-663X); Lewenstein, Maciej ORCID logo; Johnson, Allan Stewart (ORCID: 0000-0002-0711-708X)
Publisher CORA.Repositori de Dades de Recerca
Contributor Lewenstein, Maciej; Fundació Institut de Ciències Fotòniques
Publication Year 2025
Funding Reference Agencia Estatal de Investigación PID2022-137817NA-I00 ; European Research Council NOQIA ; Agencia Estatal de Investigación PGC2018-0910.13039/501100011033 ; Agencia Estatal de Investigación CEX2019-000910-S/10.13039/501100011033 ; Agencia Estatal de Investigación EUR2022-134052 ; Agencia Estatal de Investigación PID2019-106901GB-I00 ; Agencia Estatal de Investigación PID2022-139099NB-I00 ; Agencia Estatal de Investigación PRTR-C17.I1 ; Agencia Estatal de Investigación FPI ; Agencia Estatal de Investigación PCI2019-111828-2 ; Agencia Estatal de Investigación PCI2022-132919 ; European Union's Horizon 2020 101017733 ; Ministerio de transformación Digital y de la Función Público Quantum Spain ; European Union NextGenerationEU ; Fundació Cellex ; Fundació Mir-Puig ; Generalitat de Catalunya CERCA ; Agència de Gestió d'Ajuts Universitaris i de Recerca 2021 SGR 01452 ; Generalitat de Catalunya U16-011424 ; Barcelona Supercomputing Center MareNostrum FI-2023-1-0013 ; EU Quantum Flagship PASQuanS2.1 ; EU Quantum Flagship 101113690 ; EU Horizon 2020 899794 ; EU Horizon Europe 101080086–NeQST ; Fundació Institut de Ciències Fotòniques QuantumGaudi ; European Union's Horizon 2020 847648 ; “La Caixa” CF/BQ/PR23/11980043 ; La Caixa Foundation 100010434 ; Joan Oró Fellowship 2024FI-200017 ; Ramón y Cajal Program RYC2021-032392-I ; Ministerio de Ciencia, Innovación y Universidades CEX2020-001039-S
Rights CC BY-NC-ND 4.0; info:eu-repo/semantics/openAccess; http://creativecommons.org/licenses/by-nc-nd/4.0
OpenAccess true
Contact Lewenstein, Maciej (Fundació Institut de Ciències Fotòniques)
Representation
Resource Type Simulation data; Dataset
Format application/pdf; text/plain
Size 251488; 6845
Version 1.0
Discipline Natural Sciences; Physics
Spatial Coverage Castellsdefels, Catalonia, Spain