QENS analysis of industrially relevant small pore zeolites

DOI

NOx emissions from the energy and transport sectors represent a major hazard to human health and this has been the focus of significant industrial and academic research. One of the important processes in the armoury available for emissions control from vehicles, large and small, power stations, ships, trains and non-road machinery is the selective catalytic reduction reaction (SCR), in which a reductant such as ammonia, urea or hydrocarbon fuel, is injected into the exhaust to reduce the NO and NO2 (NOx) to harmless nitrogen. Copper supported on a zeolite have proven to be extremely active for SCR, and also demonstrate excellent long term stability, and are therefore often the prime choice for use in the catalytic SCR system. For these initial experiments we wish to investigate how the presence of copper and the shape of the zeolite modifies the diffusion of ammonia.

Identifier
DOI https://doi.org/10.5286/ISIS.E.63530347
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/63530347
Provenance
Creator Dr Ian Silverwood; Professor Richard Catlow; Dr Paul Collier; Dr Misbah Sarwar; Professor Stewart Parker; Dr Alexander O'Malley; Dr Andrew York; Miss Loredana Mantarosie; Dr Iain Hitchcock; Dr Sheena Hindocha
Publisher ISIS Neutron and Muon Source
Publication Year 2018
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Chemistry; Natural Sciences
Temporal Coverage Begin 2015-10-07T08:00:00Z
Temporal Coverage End 2015-10-13T08:00:00Z