Atomic structure of mercury iodide and mercury chalcohalide liquids

DOI

Optical applications of chalcogenide glasses need a wide transparency window. Promising glass systems include HgI2. Our recent studies of the yHgI2 (1-y)As2X3 glasses, where X = S, Se, have shown for the first time a significant difference in the mercury local coordination. The sulphide glasses are molecular systems with linear HgI2 molecules incorporated within the AsS3/2 glass network. The selenide glasses are polymeric with [HgIt(Ib)2/2]n chains. The trigonal mercury coordination is unusual in mercury iodides. Two different Hg-I NN coordination in the glass suggest molecular or polymeric structure in the S- or Se-based melt and possibly a liquid-liquid transition in pure HgI2 melt similar to the lambda-transition in liquid sulphur. The proposed experiment is aimed to clarify these hypotheses.

Identifier
DOI https://doi.org/10.5286/ISIS.E.49913816
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/49913816
Provenance
Creator Professor Eugene Bychkov; Dr Mariana Milochova; Dr Alex Hannon
Publisher ISIS Neutron and Muon Source
Publication Year 2017
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2014-06-02T23:00:00Z
Temporal Coverage End 2014-06-07T23:00:00Z