Fate and speciation of antimony during pyrite formation at low temperature

DOI

The geochemical behavior of Sb under reducing conditions is closely linked to the formation of digenetic iron sulfides. Since very few data is currently available on Sb speciation in such minerals, including pyrite (FeS2) ubiquitously found in surface environments, we aim at obtaining molecular scale information by performing XANES/EXAFS measurements at the Sb K-edge (30,491 eV) on synthetic FeS and FeS2 samples representative of continental sedimentary surface environments. Redox and structural information gained from XAS spectroscopy will be used together with Sb concentrations in solutions (ICP-MS), and with XRD measurement. such information is crucial to uncover the steps of Sb biogeochemical cycle in reducing surface environments and to propose conceptual models for Sb speciation in soil and sedimentary reservoirs.

Identifier
DOI https://doi.org/10.15151/ESRF-ES-2043620282
Metadata Access https://icatplus.esrf.fr/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatplus.esrf.fr:inv/2043620282
Provenance
Creator Lali CARRIERE; Mathieu CHASSE; Areej ADRA ORCID logo; Pierre LE PAPE (ORCID: 0000-0002-8100-936X); Guillaume MORIN; Olivier MATHON; Myriam BOUDIEB
Publisher ESRF (European Synchrotron Radiation Facility)
Publication Year 2028
Rights CC-BY-4.0; https://creativecommons.org/licenses/by/4.0
OpenAccess true
Representation
Resource Type Data from large facility measurement; Collection
Discipline Particles, Nuclei and Fields