Study of Fe and V speciation in the glass network of new vitrified EAF-slags to improve their use in low CO2 cements

DOI

Most low-CO2 cements use ground-granulated blast-furnace slag (GGBS), a Ca-Mg-Al-Si-glass generated as a by-product from iron-making. However, this resource is to become scarce in Europe with the transition of steel industry towards electrified production using directly reduced iron (DRI) and electric arc furnaces (EAF). Vitrification of the new EAF-slags will make them usable as cementitious material similar to GGBS. These new slags, are likely to contain higher amounts of Fe and V than traditional GGBS. The incorporation of Fe in the glass-network will affect its cementitious reactivity, depending on amount, redox state and other ions present. The presence of trace metals such as V represents a further hindrance to cementitious reactivity and their leaching behavior depends on their role in the glass network. Here, we propose to use XANES measurements in combination with µ-XRF to clarify the distribution and speciation of Fe and V in complex, synthetic, slag-glasses with compositions

Identifier
DOI https://doi.org/10.15151/ESRF-ES-2107743366
Metadata Access https://icatplus.esrf.fr/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatplus.esrf.fr:inv/2107743366
Provenance
Creator Thomas WATTEZ ORCID logo; Anna SOKOL; Katharina SCHRAUT ORCID logo; Simon BLOTEVOGEL ORCID logo; JULIEN COUTURIER (ORCID: 0000-0002-3807-457X); Astrid AVELLAN ORCID logo; Mariacristina BIANCO
Publisher ESRF (European Synchrotron Radiation Facility)
Publication Year 2028
Rights CC-BY-4.0; https://creativecommons.org/licenses/by/4.0
OpenAccess true
Representation
Resource Type Data from large facility measurement; Collection
Discipline Particles, Nuclei and Fields