Operando X-ray Diffraction Of Graphite Co-intercalation with Alkali Metals and Small Molecules

DOI

Graphite is an extensively investigated material within battery research, and it is still considered the benchmark anode for Li-ion batteries (LIBs) ever since its first commercialization, over 30 years ago. However, its application in Na-ion batteries (NIBs) remains limited due to its poor intercalation properties to form a binary graphite intercalation compounds (b-GIC) of NaCx composition. More recently an approach to circumvent this issue was demonstrated, that is to intercalate solvated alkali metals to form ternary graphite intercalation compounds (t-GIC) known as “co-intercalation” phenomenon. With this work we aim to explore this phenomenon with high time resolution to understand in detail what are the stage structures and stacking sequences of graphite during co-intercalation with different alkali metal ions and solvents.

Identifier
DOI https://doi.org/10.15151/ESRF-ES-2376080690
Metadata Access https://icatplus.esrf.fr/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatplus.esrf.fr:inv/2376080690
Provenance
Creator Alexey KOPOSOV ORCID logo; Amalie SKURTVEIT ORCID logo; Vadim DIADKIN ORCID logo; Valeria ARMENDARIZ CABRAL
Publisher ESRF (European Synchrotron Radiation Facility)
Publication Year 2029
Rights CC-BY-4.0; https://creativecommons.org/licenses/by/4.0
OpenAccess true
Representation
Resource Type Data from large facility measurement; Collection
Discipline Particles, Nuclei and Fields