Replication Data for: Chirped pulse control over the melting of superconductors

DOI

Strong field terahertz pulses are increasingly used to excite and control quantum materials at the ultrafast timescale. They have found widespread application by enabling direct addressing of the superconducting gap or Josephson resonances and are essential in Higgs spectroscopy. Large non-linear optical signals can be induced by the strong coupling of the THz and superconducting degrees of freedom. However, far less attention has been paid to the strong bidirectional coupling between field and material this implies. Here, we use the framework of the time-dependent Ginzburg-Landau equations to study the full field and material evolution of a superconductor driven by strong field terahertz pulses. We find that at high field strengths, the backreaction of the superconductor induces large changes to the driving pulse, which in turn leads to a runaway melting of the superconducting condensate. This results in a surprisingly large sensitivity to the initial driving pulse chirp, enabling these purely dynamical changes to produce order of magnitude differences in the level of melting. We also find large-scale spectral shifting of the driving pulse to occur in just a few hundred nanometers of propagation through a superconductor. We attribute these effects to an inverse plasma redshift, in which the driving field breaks Cooper pairs and decreases the free-electron mobility, analogous to reducing the density of a plasma.

Identifier
DOI https://doi.org/10.34810/DATA2159
Related Identifier IsSupplementTo https://doi.org/10.1103/PhysRevB.111.064513
Metadata Access https://dataverse.csuc.cat/oai?verb=GetRecord&metadataPrefix=oai_datacite&identifier=doi:10.34810/DATA2159
Provenance
Creator Recasens, Maria ORCID logo; Kasper, Valentin (ORCID: 0000-0001-7687-663X); Lewenstein, Maciej ORCID logo; Johnson, Allan Stewart (ORCID: 0000-0002-0711-708X)
Publisher CORA.Repositori de Dades de Recerca
Contributor Lewenstein, Maciej; Fundació Institut de Ciències Fotòniques
Publication Year 2025
Funding Reference https://ror.org/00k4n6c32 NOQIA ; https://ror.org/00k4n6c32 101017733 ; https://ror.org/00k4n6c32 NextGenerationEU ; https://ror.org/01bg62x04 2021 SGR 01452 ; https://ror.org/00k4n6c32 ; https://ror.org/00k4n6c32 899794 ; https://ror.org/00k4n6c32 101080086–NeQST ; https://ror.org/00k4n6c32 847648 ; https://ror.org/03zhx9h04 CF/BQ/PR23/11980043 ; https://ror.org/03zhx9h04 100010434
Rights CC BY-NC-ND 4.0; info:eu-repo/semantics/openAccess; http://creativecommons.org/licenses/by-nc-nd/4.0
OpenAccess true
Contact Lewenstein, Maciej (Fundació Institut de Ciències Fotòniques)
Representation
Resource Type Simulation data; Dataset
Format application/pdf; text/plain
Size 251488; 6845
Version 1.0
Discipline Natural Sciences; Physics
Spatial Coverage Castellsdefels, Catalonia, Spain