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RF-muSR in the gas phase: the muoniated ethyl radical
Radio-frequency muon spin resonance is an exceptional technique for studying free radicals, but it has not been applied to study radicals in the gas phase. In a previous... -
Investigating magneto-superconductivity of CeO0.5F0.5BiS2 and Ce0.5Sr0.5FBiS2
In this proposal we plan to investigate the anomalous magnetism of Ce in recently discovered CeO0.5F0.5BiS2 and Sr0.5Ce0.5FBiS2 magneto-superconductors. The proposed compounds... -
Artificial [FeFe]-Hydrogenases and Muon Spectroscopy
Preliminary measurements of [FeFe]-hydrogenase model complexes were made in a previous experiment using EMU (RB 1010177). The results were interpreted in combination with DFT... -
Ultrafast motion of molecular rotors in metal-organic frameworks: a muon-spin...
In recent years, amphidynamic crystals have gained more and more attention as a state of matter somehow intermediate between solids and liquids. In fact, although these systems... -
Probing the magnetic ground state in one dimensional magnetic systems Ba3CrS5...
Most of the one dimensional spin chain compounds are antiferromagnetic with a rich magnetic phase diagram due to the magnetic frustration. We have synthesized Ba3CrS5 and... -
Electron Spin Relaxation Measurements of P3HS
Using muon spin relaxation and ALC resonance spectroscopy the electron spin relaxation and mobility of the polymer P3HS will be measured as a function of temperature. The... -
Characterizing neutral and diamagnetic Mu in beta-Ga2O3
We propose a series of LF-MuSR measurements to complete a study on the neutral and diamagnetic muonium (Mu) states in single-crystal beta-Ga2O3 where Mu is being used as an... -
Geometrical frustration induced magnetism in single crystal of CeIrSn: A Muon...
The quasi-kagome Kondo lattice CeRhSn exhibits quantum criticality induced by geometrical frustration. Divergent Grüneisen ratios provide evidence for a zero-field QCP. The... -
Muon Spin Relaxation and ALC Resonance in Magnetic and non-Magnetic Oxalate S...
Repolarisation and level crossing resonance will be studied for several different oxalate compounds where muon radical states are known to be formed. Such compounds form a... -
Repolarization of Radicals in Liquids
The recovery of the muon polarization in a longitudinal magnetic field has been used to obtain the muon hfcs of organic radicals. In pure benzene there is a single step in the... -
ALC muon spectroscopy of antioxidants
In a previous experiment (RB910492) we have made preliminary measurements of the rates of addition of muonium to vitamins C and E, as suggested by the ISIS panel. These rates... -
Validating a new theoretical method for predicting the HFC of small molecular...
ALC is the best technique to characterize muoniated radicals, that are produced by muonium bonding to unsaturated bonds in molecules. Good agreement between data from ALC and... -
Muon level-crossing resonances as a probe for studying antiferromagnets at pu...
We propose a set of measurements using the HiFi spectrometer in which muon level-crossing resonances are used to probe the internal field inside antiferromagnets in which the... -
Muonium in rare-earth sesquioxides
We propose to characterize the basic muonium/hydrogen configurations in selected rare-earth sesquioxides with the basic crystallographic structures: neodymium oxide (hexagonal A... -
Tunneling and relaxation of the magnetization in Mn6 single molecule magnet
The Mn6 single molecule magnet shows to date the highest anisotropy barrier for a transition metal cluster. Low lying excited states in the energy level diagram of the molecule... -
Models of the [FeFe]-hydrogenase active site: raising the symmetry
The [FeFe]-hydrogenase enzymes are some of the best catalysts know for generating hydrogen. We have an ongoing programme to understand how their chemistry works, and to... -
Muon spin relaxation studies of KTCNQ and related compounds
Potassium tetracyanoquinodimenthane (KTCNQ) undergoes a spin-Peierls (SP) transition at 396K where a transformation from uniform to dimerised TCNQ- molecules in 1D columns... -
RF MuSR in the gas phase: the Search for a Radical State
The main spectroscopic technique for studying radicals in solids and liquids, ESR, cannot usually be used to study radicals of more than 3-5 atoms in the gas phase due to strong... -
Muon response to changes in the charge distribution of the components of a co...
We plan to confirm that the change in asymmetry on resonance in the ALC spectra seen in the subject complex dielectric during the previous rapid access proposal (RB1900028) is a... -
Organometallic Radicals
Avoided level crossing muon spin resonance (ALC-muSR) is an exceptional tool for determining the structure and probing the dynamics of radicals but there have been only a few...
