Entropy Scaling Laws in Self Propelled Glass Formers

Here we probe a glass forming liquid composed of self- propelled “active” particles and show that increasing the duration of self-propulsion makes the pair excess entropy negatively larger. The associated reduction in the number of accessible configurations per particle leads to a reduction in self- diffusivity. At moderate supercooling, the self-diffusivity is Arrhenius and in a reduced form obeys a Dzugutov like scaling law, directly yielding us a pair excess entropy that is inversely proportional to the effective temperature. In the strongly super-cooled regime, Dzugutov law does not apply and we observe that, the pair excess entropy shows a non-Arrhenius (power law) dependence on the effective temperature with an exponent that depends on the self propulsion time of the active particles.

Identifier
DOI https://doi.org/10.17632/7jkb7cyndm.1
PID https://nbn-resolving.org/urn:nbn:nl:ui:13-kp-20w1
Metadata Access https://easy.dans.knaw.nl/oai?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:easy.dans.knaw.nl:easy-dataset:219715
Provenance
Creator C N, S
Publisher Data Archiving and Networked Services (DANS)
Contributor SACHIN C N
Publication Year 2021
Rights info:eu-repo/semantics/openAccess; License: http://creativecommons.org/licenses/by/4.0; http://creativecommons.org/licenses/by/4.0
OpenAccess true
Representation
Resource Type Dataset
Discipline Other